Investigation of the effect of electron beam irradiation on the structural and transport properties of half doped Nd 0.5 Sr 0.5 MnO 3 manganites

Pronita Chettri, Utpal Deka, Ashok Rao, G. S. Okram, Vikash Chandra Petwal, Vijay Pal Verma, Jishnu Dwivedi, Riya Thomas, B. S. Nagaraja

Research output: Contribution to journalArticle

Abstract

A systematic investigation on the effect of electron beam irradiation on the structural, electrical properties and thermopower of half doped Nd 0.5 Sr 0.5 MnO 3 manganites is presented in this report. Elemental analysis of the samples through Energy Dispersive X-ray Spectroscopy (EDS) confirm the desired stoichiometry. Rietveld refinement of the X Ray diffraction data reveals that the samples are single phased. Further, no change in crystal structure or symmetry is observed as an after-effect of electron beam radiation. The samples exhibit insulating behaviour in the entire temperature range 10–300 K. Though the resistivity value changes as a result of electron beam irradiation but the insulating behaviour is unaffected. It is validated from both resistivity as well as thermopower analysis that small polarons are responsible for conduction in the high temperature region. On the contrary, variable range hopping is responsible for the conduction mechanism at low temperatures. The absolute value of thermopower is observed to decrease with increasing dose of electron beam. Moreover, thermopower data indicates n-type conductivity for the samples under investigation.

Original languageEnglish
Pages (from-to)220-227
Number of pages8
JournalPhysica B: Condensed Matter
Volume560
DOIs
Publication statusPublished - 01-05-2019

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Manganites
Thermoelectric power
Transport properties
Structural properties
Electron beams
transport properties
Irradiation
electron beams
irradiation
conduction
Polarons
electrical resistivity
Rietveld refinement
Crystal symmetry
polarons
Stoichiometry
Temperature
Energy dispersive spectroscopy
stoichiometry
Electric properties

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Electrical and Electronic Engineering

Cite this

Chettri, Pronita ; Deka, Utpal ; Rao, Ashok ; Okram, G. S. ; Chandra Petwal, Vikash ; Verma, Vijay Pal ; Dwivedi, Jishnu ; Thomas, Riya ; Nagaraja, B. S. / Investigation of the effect of electron beam irradiation on the structural and transport properties of half doped Nd 0.5 Sr 0.5 MnO 3 manganites. In: Physica B: Condensed Matter. 2019 ; Vol. 560. pp. 220-227.
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Investigation of the effect of electron beam irradiation on the structural and transport properties of half doped Nd 0.5 Sr 0.5 MnO 3 manganites. / Chettri, Pronita; Deka, Utpal; Rao, Ashok; Okram, G. S.; Chandra Petwal, Vikash; Verma, Vijay Pal; Dwivedi, Jishnu; Thomas, Riya; Nagaraja, B. S.

In: Physica B: Condensed Matter, Vol. 560, 01.05.2019, p. 220-227.

Research output: Contribution to journalArticle

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AU - Chettri, Pronita

AU - Deka, Utpal

AU - Rao, Ashok

AU - Okram, G. S.

AU - Chandra Petwal, Vikash

AU - Verma, Vijay Pal

AU - Dwivedi, Jishnu

AU - Thomas, Riya

AU - Nagaraja, B. S.

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N2 - A systematic investigation on the effect of electron beam irradiation on the structural, electrical properties and thermopower of half doped Nd 0.5 Sr 0.5 MnO 3 manganites is presented in this report. Elemental analysis of the samples through Energy Dispersive X-ray Spectroscopy (EDS) confirm the desired stoichiometry. Rietveld refinement of the X Ray diffraction data reveals that the samples are single phased. Further, no change in crystal structure or symmetry is observed as an after-effect of electron beam radiation. The samples exhibit insulating behaviour in the entire temperature range 10–300 K. Though the resistivity value changes as a result of electron beam irradiation but the insulating behaviour is unaffected. It is validated from both resistivity as well as thermopower analysis that small polarons are responsible for conduction in the high temperature region. On the contrary, variable range hopping is responsible for the conduction mechanism at low temperatures. The absolute value of thermopower is observed to decrease with increasing dose of electron beam. Moreover, thermopower data indicates n-type conductivity for the samples under investigation.

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